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By W.G. Frankenburg, V.I. Komarewsky, E.K. Rideal (Eds.)
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Additional resources for Advances in Catalysis, Vol. 6
This expression, in its integrated form, was derived exactly by Ward and Tordai (26), and tested experimentally in various ways. Use of radioactive tracers (27), for example, has made possible direct checks. The method involves a tracer element emitting very soft prays. Only those atoms in or very near the interface contribute to the radioactivity just above the surface; TABLE I1 Concn. of Al+S in bulk, expressed in moles liter-' 10-4 M 10-6 M 10-6 M 10-7 M 10-8 M Time for monolayer of stearic acid t o be converted into the A1 sdt, calc.
05 is calculated Here 1 / is for water a t 25°C. The concentration, c, is expressed in moles per liter. The magnitude of the electrical potential at the interface can be estimated in several ways. One of these involves the adsorption of dyes. Donnan equations, a-loA 0 I I I I I 1 2 3 4 I 5 Added NaCl (normality) FIG. 19. CO~-. clectrical charge. This repels the similarly charged hydrolytic hydroxyl ions. The height of this electrical repulsive barrier is reduced greatly by any “neutral” salts (Davies and Rideal, 21).
K is in liter mol.? -l units. as in the case of oleic acid, as the film is compressed the molecules are packed more closely in the surface, and the double bonds are forced out of the interface, as shown respectively in Figs. 2 and 1. To effect this change, work is done on the molecules by the film pressure n and also by any cohesive forces between the hydrocarbon chains. Since the forces are apparently very small for the particular case of triolein films the third factor above may be neglected.
Advances in Catalysis, Vol. 6 by W.G. Frankenburg, V.I. Komarewsky, E.K. Rideal (Eds.)